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Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1358-2

摘要：

• Microbes enhance denitrification under varying DO concentrations and SIF dosages.

关键词： Scrap iron filing     Nitrate removal     Phosphate removal     Mixed culture denitrification     Zero valent iron    

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Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1454-y

摘要：

Membrane bioreactor achieved mercury removal using nitrate as an electron acceptor.

关键词： Mercury removal     Oxygen     Ferrous sulfide     Transformation of mercury     Microbial community    

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Electrochemical removal of nitrate in industrial wastewater

Dong Xu, Yang Li, Lifeng Yin, Yangyuan Ji, Junfeng Niu, Yanxin Yu

《环境科学与工程前沿（英文）》 2018年 第12卷 第1期 doi: 10.1007/s11783-018-1033-z

摘要： A number of recent studies have demonstrated that electrochemical technologies, including electroreduction (ER), electrocoagulation (EC), and electrodialysis (ED), are effective in nitrate elimination in wastewater due to their high reactivity. To obtain the maximal elimination efficiency and current efficiency, many researchers have conducted experiments to investigate the optimal conditions (i.e., potential, current density, pH value, plate distance, initial nitrate concentration, electrolyte, and other factors) for nitrate elimination. The mechanism of ER, EC and ED for nitrate removal has been fully elucidated. The ER mechanism of nitrate undergoes electron transfer and hydrogenation reduction. The EC pathways of nitrate removal include reduction, coagulation and flotation. The ED pathways of nitrate include redox reaction and dialysis. Although the electrochemical technology can remove nitrate from wastewater efficiently, many problems (such as relatively low selectivity toward nitrogen, sludge production and brine generation) still hinder electrochemical treatment implementation. This paper critically presents an overview of the current state-of-the-art of electrochemical denitrification to enhance the removal efficiency and overcome the shortages, and will significantly improve the understanding of the detailed processes and mechanisms of nitrate removal by electrochemical treatment and provide useful information to scientific research and actual practice.

关键词： Nitrate removal     Electroreduction     Electrocoagulation     Electrodialysis    

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Simultaneous enhanced ammonia and nitrate removal from secondary effluent in constructed wetlands using

《环境科学与工程前沿（英文）》 2023年 第18卷 第4期 doi: 10.1007/s11783-024-1807-4

摘要：

● MnO2/PCL composite material (MPCM) enhances ammonia and nitrate removal in CWs.

关键词： Constructed wetland     Nitrogen removal     Manganese redox     Polycaprolactone     Nitrous oxide    

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Erratum to: Electrochemical removal of nitrate in industrial wastewater

Dong Xu, Yang Li, Lifeng Yin, Yangyuan Ji, Junfeng Niu, Yanxin Yu

《环境科学与工程前沿（英文）》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1038-7

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Removal of ammonium and nitrate through Anammox and FeS-driven autotrophic denitrification

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1674-4

摘要：

● Simultaneous NH4+/NO3– removal was achieved in the FeS denitrification system

关键词： Anammox     Denitrification     FeS     NH4+/NO3−     Sulfammox    

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LYX: A novel aerobic bacterium with advantage of removing nitrate high effectively by assimilation and

Yuxin Li, Jiayin Ling, Pengcheng Chen, Jinliang Chen, Ruizhi Dai, Jinsong Liao, Jiejing Yu, Yanbin Xu

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1349-3

摘要： Abstract • Pseudomonas mendocina was first reported for aerobic nitrate removal. • It removed 90% of NO3−-N in 24 h under aerobic conditions. • This strain converted NO3−-N to bio-nitrogen (37.9%) and gaseous nitrogen (49.7%). • Inoculation of this strain increased sludge denitrification rate by 4.3 times. The problem of nitrate accumulation in aerobic tank and total nitrogen excessive discharge in effluent was very common in traditional livestock and poultry farming wastewater treatment systems owing to the lengthy process flow and low process control level. A strain LYX of aerobic bacterium was isolated from the activated sludge of a wastewater treatment system in a pig farm, which could remove nitrate effectively in aerobic tank and was identified Pseudomonas mendocina by 16S rRNA sequencing. Under the condition of nitrate as the sole nitrogen source, this strain removed over 90% of NO3−-N with an initial concentration of 110 mg/L under aerobic conditions within 48 hours. Among them, 37.9% of NO3−-N was assimilated into Bio-N, about 51.9% was reduced to gaseous nitrogen and less than 0.5% of nitrogen was replaced by NO2−-N and NH4+-N, 9.7% NO3−-N remained in the effluent at the end. At the same time, four key genes (napA, nirK, norB and nosZ) related to nitrate nitrogen removal were expressed during the denitrification process of P. mendocina LYX, in which the transcription level of the indicator genes of this aerobic denitrifying bacterium (napA) was the highest. In addition, it was found with the 15N tracer technique that inoculation of this strain on sludge increased the amount of nitrogen loss from 9.26 nmol N/(g·h) to 23.835 nmol N/(g·h). Therefore, P. medocina LYX is a potential bioagent for advanced nitrogen removal by assimilating and reducing nitrate simultaneously in aerobic tanks.

关键词： Pseudomonas mendocina     Aerobic nitrate removal     15N tracing technique     Denitrification assimilatively and disimilatively     Aerobic denitrifying genes    

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基于元分析揭示全球尺度下反硝化反应器中基质材料对硝态氮去除的显著影响 Review

范豫川, 庄杰, Michael Essington, Sindhu Jagadamma, John Schwartz, Jaehoon Lee

《工程（英文）》 2023年 第21卷 第2期   页码 214-226 doi: 10.1016/j.eng.2022.08.017

摘要：

反硝化生物反应器（DNBR）被广泛用于减少农业废水中过量的硝态氮。其性能取决于基质的物理和化学性质。在以前的研究中，已经对一部分常见基质做了总结。然而，很少有研究尝试确定基质类型在硝态氮去除中起作用的一般模式。本研究利用从63 篇同行评议文章中收集的数据总结了41 种基质类型，包括219 个独立DNBR单元。基质分为四类：①天然碳（NC），如木屑；②非天然碳（NNC），如可生物降解聚合物[如聚己内酯（PCL）和废品（如纸板）]；③无机材料（IM），如非碳材料（如氧化铁）；④复合材料（MM），如上述材料的混合物。通过对硝态氮去除速率[NRR，氮去除（g∙m‒3∙d‒1）]和硝态氮去除效率（NRE, %）的元分析，对这些材料进行比较和评估。本文综合阐述了基质效果（NRR和NRE）、潜在机理、污染交换和成本分析。我们的分析表明，木屑和玉米芯是NC中最具成本效益的基质。对比所有参与研究的基质，我们建议将MM作为最优基质，尤其是具有很大的改进空间的基于木屑和玉米芯的基质。该分析有助于优化DNBR的设计，以满足使用者对环境、经济和实用的需求。

关键词： 反硝化生物反应器     基质     硝酸盐去除     元分析     环境影响     成本分析    

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Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

《能源前沿（英文）》 doi: 10.1007/s11708-023-0908-2

摘要： The Haber-Bosch process is the most widely used synthetic ammonia technology at present. Since its invention, it has provided an important guarantee for global food security. However, the traditional Haber-Bosch ammonia synthesis process consumes a lot of energy and causes serious environmental pollution. Under the serious pressure of energy and environment, a green, clean, and sustainable ammonia synthesis route is urgently needed. Electrochemical synthesis of ammonia is a green and mild new method for preparing ammonia, which can directly convert nitrogen or nitrate into ammonia using electricity driven by solar, wind, or water energy, without greenhouse gas and toxic gas emissions. Herein, the basic mechanism of the nitrogen reduction reaction (NRR) to ammonia and nitrate reduction reaction (NO3− RR) to ammonia were discussed. The representative approaches and major technologies, such as lithium mediated electrolysis and solid oxide electrolysis cell (SOEC) electrolysis for NRR, high activity catalyst and advanced electrochemical device fabrication for NO3 − RR and electrochemical ammonia synthesis were summarized. Based on the above discussion and analysis, the main challenges and development directions for electrochemical ammonia synthesis were further proposed.

关键词： electrochemical ammonia synthesis     nitrogen     nitrate     nitrogen reduction reaction (NRR) to ammonia     nitrate reduction reaction (NO–3 RR)    

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Rapid and long-effective removal of broad-spectrum pollutants from aqueous system by ZVI/oxidants

Sana Ullah, Xuejun Guo, Xiaoyan Luo, Xiangyuan Zhang, Siwen Leng, Na Ma, Palwasha Faiz

《环境科学与工程前沿（英文）》 2020年 第14卷 第5期 doi: 10.1007/s11783-020-1268-3

摘要： Abstract • The coupling of oxidants with ZVI overcome the impedance of ZVI passive layer. • ZVI/oxidants system achieved fast and long-effective removal of contaminants. • Multiple mechanisms are involved in contaminants removal by ZVI/oxidant system. • ZVI/Oxidants did not change the reducing property of ORP in the fixed-bed system. Zero-valent iron (ZVI) technology has recently gained significant interest in the efficient sequestration of a wide variety of contaminants. However, surface passivation of ZVI because of its intrinsic passive layer would lead to the inferior reactivity of ZVI and its lower efficacy in contaminant removal. Therefore, to activate the ZVI surface cheaply, continuously, and efficiently is an important challenge that ZVI technology must overcome before its wide-scale application. To date, several physical and chemical approaches have been extensively applied to increase the reactivity of the ZVI surface toward the elimination of broad-spectrum pollutants. Nevertheless, these techniques have several limitations such as low efficacy, narrow working pH, eco-toxicity, and high installation cost. The objective of this mini-review paper is to identify the critical role of oxygen in determining the reactivity of ZVI toward contaminant removal. Subsequently, the effect of three typical oxidants (H2O2, KMnO4, and NaClO) on broad-spectrum contaminants removal by ZVI has been documented and discussed. The reaction mechanism and sequestration efficacies of the ZVI/oxidant system were evaluated and reviewed. The technical basis of the ZVI/oxidant approach is based on the half-reaction of the cathodic reduction of the oxidants. The oxidants commonly used in the water treatment industry, i.e., NaClO, O3, and H2O2, can be served as an ideal coupling electron receptor. With the combination of these oxidants, the surface corrosion of ZVI can be continuously driven. The ZVI/oxidants technology has been compared with other conventional technologies and conclusions have been drawn.

关键词： Zero-Valent Iron (ZVI)     Oxidants     Heavy Metals (HMs)     Metalloids     Nitrate     Phosphate    

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Optimization of denitrifying phosphorus removal in a pre-denitrification anaerobic/anoxic/post-aeration

Weihua Zhao, Meixiang Wang, Jianwei Li, Yu Huang, Baikun Li, Cong Pan, Xiyao Li, Yongzhen Peng

《环境科学与工程前沿（英文）》 2018年 第12卷 第5期 doi: 10.1007/s11783-018-1084-1

摘要：

A novel two sludge pre-A2NSBR system was developed.

Advanced N and P removal was optimized to treat real domestic wastewater.

Nitrifiers and PAOs were enriched with 19.41% and 26.48%, respectively.

Acetate was demonstrated as the high-quality carbon source type.

关键词： Denitrifying phosphorus removal     C/N ratio     Nitrate recycling     Carbon source type     Biological nutrient removal     Pre-A2NSBR system    

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Nitrate removal to its fate in wetland mesocosm filled with sponge iron: Impact of influent COD/N ratio

Zhihao Si, Xinshan Song, Xin Cao, Yuhui Wang, Yifei Wang, Yufeng Zhao, Xiaoyan Ge, Awet Arefe Tesfahunegn

《环境科学与工程前沿（英文）》 2020年 第14卷 第1期 doi: 10.1007/s11783-019-1183-7

摘要： CW-Fe allowed a high-performance of NO3‒-N removal at the COD/N ratio of 0. Higher COD/N resulted in lower chem-denitrification and higher bio-denitrification. The application of s-Fe0 contributed to TIN removal in wetland mesocosm. s-Fe0 changed the main denitrifiers in wetland mesocosm. Sponge iron (s-Fe0) is a porous metal with the potential to be an electron donor for denitrification. This study aims to evaluate the feasibility of using s-Fe0 as the substrate of wetland mesocosms. Here, wetland mesocosms with the addition of s-Fe0 particles (CW-Fe) and a blank control group (CW-CK) were established. The NO3‒-N reduction property and water quality parameters (pH, DO, and ORP) were examined at three COD/N ratios (0, 5, and 10). Results showed that the NO3‒-N removal efficiencies were significantly increased by 6.6 to 58.9% in the presence of s-Fe0. NH4+-N was mainly produced by chemical denitrification, and approximately 50% of the NO3‒-N was reduced to NH4+-N, at the COD/ratio of 0. An increase of the influent COD/N ratio resulted in lower chemical denitrification and higher bio-denitrification. Although chemical denitrification mediated by s-Fe0 led to an accumulation of NH4+-N at COD/N ratios of 0 and 5, the TIN removal efficiencies increased by 4.5%‒12.4%. Moreover, the effluent pH, DO, and ORP values showed a significant negative correlation with total Fe and Fe (II) (P<0.01). High-throughput sequencing analysis indicated that Trichococcus (77.2%) was the most abundant microorganism in the CW-Fe mesocosm, while Thauera, Zoogloea, and Herbaspirillum were the primary denitrifying bacteria. The denitrifiers, Simplicispira, Dechloromonas, and Denitratisoma, were the dominant bacteria for CW-CK. This study provides a valuable method and an improved understanding of NO3‒-N reduction characteristics of s-Fe0 in a wetland mesocosm.

关键词： Sponge iron     Wetland mesocosm     Electronic donor     Denitrification     COD/N ratio    

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硝酸铵膨化理论研究

吕春绪

《中国工程科学》 2001年 第3卷 第9期   页码 58-63

摘要：

描述了硝酸铵膨化过程，计算与测定了其物理化学参数，研究了膨化过程的影响因素，并给出了膨化过程可能的机理。

关键词： 膨化硝酸铵     膨化理论     物理化学参数     影响因素    

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Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

《化学科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 55-58 doi: 10.1007/s11705-007-0011-y

摘要： Isolated MnO nanotubes and nanofibers were prepared very easily at a large scale with the liquid-phase catalysis method. The MnO nanotubes had dimensions of 30 50 nm (exterior diameter) and 0.2 1.0 ?m (length), approximately. The O nanofibers had dimensions of 10 30 nm (diameter) and 0.4 2.0 ?m (length), approximately. Nano-O with different microstructures including nanotubes, nanofibers and nanoparticles could be selectively synthesized by controlling the contents and proportions of potassium permanganate and ferric nitrate. Ferric nitrate was an ideal catalyst for the preparation of O nanotube/fiber. When cobalt nitrate or nickel nitrate was used as catalyst, only amorphous nano-O was synthesized. X-ray diffraction (XRD) result shows that the O nanotube has a crystalline structure different from o-O, t-O, h-O and ?-O.

关键词： different     nickel     exterior diameter     nanotube     XRD    

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New insights into the formation of ammonium nitrate from a physical and chemical level perspective

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1737-6

摘要：

● Factor analysis of ammonium nitrate formation based on thermodynamic theory.

关键词： Ammonium nitrate formation     Thermodynamic theory     Aerosol liquid water content     Source apportionment    

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标题 作者 时间 类型 操作

Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

期刊论文

Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

期刊论文

Electrochemical removal of nitrate in industrial wastewater

Dong Xu, Yang Li, Lifeng Yin, Yangyuan Ji, Junfeng Niu, Yanxin Yu

期刊论文

Simultaneous enhanced ammonia and nitrate removal from secondary effluent in constructed wetlands using

期刊论文

Erratum to: Electrochemical removal of nitrate in industrial wastewater

Dong Xu, Yang Li, Lifeng Yin, Yangyuan Ji, Junfeng Niu, Yanxin Yu

期刊论文

Removal of ammonium and nitrate through Anammox and FeS-driven autotrophic denitrification

期刊论文

LYX: A novel aerobic bacterium with advantage of removing nitrate high effectively by assimilation and

Yuxin Li, Jiayin Ling, Pengcheng Chen, Jinliang Chen, Ruizhi Dai, Jinsong Liao, Jiejing Yu, Yanbin Xu

期刊论文

基于元分析揭示全球尺度下反硝化反应器中基质材料对硝态氮去除的显著影响

范豫川, 庄杰, Michael Essington, Sindhu Jagadamma, John Schwartz, Jaehoon Lee

期刊论文

Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

期刊论文

Rapid and long-effective removal of broad-spectrum pollutants from aqueous system by ZVI/oxidants

Sana Ullah, Xuejun Guo, Xiaoyan Luo, Xiangyuan Zhang, Siwen Leng, Na Ma, Palwasha Faiz

期刊论文

Optimization of denitrifying phosphorus removal in a pre-denitrification anaerobic/anoxic/post-aeration

Weihua Zhao, Meixiang Wang, Jianwei Li, Yu Huang, Baikun Li, Cong Pan, Xiyao Li, Yongzhen Peng

期刊论文

Nitrate removal to its fate in wetland mesocosm filled with sponge iron: Impact of influent COD/N ratio

Zhihao Si, Xinshan Song, Xin Cao, Yuhui Wang, Yifei Wang, Yufeng Zhao, Xiaoyan Ge, Awet Arefe Tesfahunegn

期刊论文

硝酸铵膨化理论研究

吕春绪

期刊论文

Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

期刊论文

New insights into the formation of ammonium nitrate from a physical and chemical level perspective

期刊论文